Publications

Science Advances (2022)

Optical-field sampling techniques provide direct access to the electric field of visible and near-infrared light. The existing methods achieve the necessary bandwidth using highly nonlinear light-matter interaction that involves ionization of atoms or generation of charge carriers in solids. We demonstrate an alternative, all-optical approach for measuring electric fields of broadband laser pulses, which offers an advantage in terms of sensitivity and signal-to-noise ratio and extends the detection bandwidth of optical methods to the petahertz domain.

Nature Communications (2022)

Light-field driven charge motion links semiconductor technology to electric fields with attosecond temporal control. Motivated by ultimate-speed electron-based signal processing, strong-field excitation has been identified viable for the ultrafast manipulation of a solid’s electronic properties but found to evoke perplexing post-excitation dynamics. Here, we report on single-photon-populating the conduction band of a wide-gap dielectric within approximately one femtosecond. We control the subsequent Bloch wavepacket motion with the electric field of visible light. The resulting current allows sampling optical fields and tracking charge motion driven by optical signals. Our approach utilizes a large fraction of the conduction-band bandwidth to maximize operating speed. We identify population transfer to adjacent bands and the associated group velocity inversion as the mechanism ultimately limiting how fast electric currents can be controlled in solids. Our results imply a fundamental limit for classical signal processing and suggest the feasibility of solid-state optoelectronics up to 1 PHz frequency.

Nature Communications (2022)

The measurement and control of light field oscillations enable the study of ultrafast phenomena on sub-cycle time scales. Electro-optic sampling (EOS) is a powerful field characterization approach, in terms of both sensitivity and dynamic range, but it has not reached beyond infrared frequencies. Here, we show the synthesis of a sub-cycle infrared-visible pulse and subsequent complete electric field characterization using EOS. The sampled bandwidth spans from 700 nm to 2700 nm (428 to 110 THz). Tailored electric-field waveforms are generated with a two-channel field synthesizer in the infrared-visible range, with a full-width at half-maximum duration as short as 3.8 fs at a central wavelength of 1.7 µm (176 THz). EOS detection of the complete bandwidth of these waveforms extends it into the visible spectral range. To demonstrate the power of our approach, we use the sub-cycle transients to inject carriers in a thin quartz sample for nonlinear photoconductive field sampling with sub-femtosecond resolution.

Nature Communications (2022)

Photoconductive field sampling enables petahertz-domain optoelectronic applications that advance our understanding of light-matter interaction. Despite the growing importance of ultrafast photoconductive measurements, a rigorous model for connecting the microscopic electron dynamics to the macroscopic external signal is lacking. This has caused conflicting interpretations about the origin of macroscopic currents. Here, we present systematic experimental studies on the signal formation in gas-phase photoconductive sampling. Our theoretical model, based on the Ramo–Shockley-theorem, overcomes the previously introduced artificial separation into dipole and current contributions. Extensive numerical particle-in-cell-type simulations permit a quantitative comparison with experimental results and help to identify the roles of electron-neutral scattering and mean-field charge interactions. The results show that the heuristic models utilized so far are valid only in a limited range and are affected by macroscopic effects. Our approach can aid in the design of more sensitive and more efficient photoconductive devices.

The International Conference on Ultrafast Phenomena (UP) 2022 (2022)

We present the generation of a supercontinuum soft-X-ray spectrum generated by high-harmonic generation driven by self-compressed 1450 nm pulses using the soliton effect. The compression of 2.8 mJ, 30 fs pulses down to sub 10-fs (supporting 7.2 fs duration) is achieved in a hollow-core fiber and delivered to the HHG target under vacuum using no additional dispersive optics.

Physical Review Letters (2021)

Multiphoton excitation of a solid by a few-cycle, intense laser pulse forms a very nonequilibrium distribution of charge carriers, where occupation probabilities do not necessarily decrease with energy. Within a fraction of the pulse, significant population inversion can emerge between pairs of valence-band states with a dipole-allowed transition between them. This population inversion leads to stimulated emission in a laser-excited solid at frequencies where the unperturbed solid is transparent. We establish the optimal conditions for observing this kind of strong-field-induced optical gain.

Nanophotonics (2021)

Strong-field photoemission from nanostructures and the associated temporally modulated currents play a key role in the development of ultrafast vacuum optoelectronics. Optical light fields could push their operation bandwidth into the petahertz domain. A critical aspect of their functionality in the context of applications is the impact of charge interaction effects. Here, we investigated the photoemission and photocurrents from nanometric tungsten needle tips exposed to carrier-envelope phase (CEP)-controlled few-cycle laser fields. We report a characteristic rapid increase in the intensity-rescaled cutoff energies of emitted electrons beyond a certain intensity value. By comparison with simulations, we identify this feature as the onset of charge-interaction dominated photoemission dynamics. Our results are anticipated to be relevant also for the strong-field photoemission from other nanostructures, including photoemission from plasmonic nanobowtie antennas used in CEP-detection and for PHz-scale devices.

Optica (2021)

The electric field waveform of a light field can be used to unlock a detailed recording of its interaction with matter, but accessing it requires a measurement with subfemtosecond temporal resolution. We demonstrate nonlinear photoconductive sampling of light fields at optical frequencies in ambient air. The resulting detection method provides broadband electric field measurement in an inexpensive setup using a self-healing medium. A direct comparison is made between detection in air and in quartz, validating the technique up to 0.7 PHz. This provides both a simple route toward field metrology and a new platform for future studies in attosecond physics without the need for complex vacuum setups or sophisticated sample preparation.

arXiv (2021)

Direct access to the electric field of light provides a subcycle view of the polarization response of matter, thus enabling sensitive metrology in physics, chemistry, and medicine. Optical-field sampling techniques take advantage of some process that lasts much less than an optical cycle of the measured light wave. Most of them rely on the generation of free electrons either by a weak extreme ultraviolet pulse or by a strong optical pulse. The ability of such techniques to detect weak signals is limited by undesirable effects associated with ionization. An alternative is all-optical methods, where the fast process is a nonlinear wave mixing. Such photonic methods may rely on extreme ultraviolet or optical pulses. They typically have better sensitivity, but smaller bandwidth. Here we propose generalized heterodyne optical-sampling techniques (GHOSTs), which overcome the bandwidth limit through controlling light-pulse waveforms.

Ludwig-Maximilians-Universität München (2021)

Fast evolving technologies require faster data processing. Modern electronics possess physical limits for computation speed. To circumvent these limits new scientific approaches are required. Light is the fastest information carrier, therefore optoelectronic light-matter interaction can be potentially employed as a method towards much faster computation. In order to exploit light-matter interactions in the attosecond temporal and petahertz spectral domains, three main conditions should be fulfilled: a) techniques capable of detecting such fast processes must be available, b) physical mechanisms with an attosecond response time should be found and characterized, c) the methodology for storing and controlling of the information by means of these fast processes should be developed. This dissertation addresses these conditions and demonstrates the applicability of optoelectronics towards attosecond and petahertz domains.